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  1. null (Ed.)
    Spontaneous parametric down conversion (PDC), in the perturbative limit, can be considered as a probabilistic splitting of one input photon into two output photons. Conversely, sum-frequency generation (SFG) implements the reverse process of combining two input photons into one. Here we show that a single-photon projective measurement in the temporal-mode basis of the output photon of a two-photon SFG process affects a generalized measurement on the input two-photon state. We describe the positive operator-valued measure (POVM) associated with such a measurement and show that its elements are proportional to the two-photon states produced by the time-reversed PDC process. Such a detection acts as a joint measurement on two photons and is thus an important component of many quantum information processing protocols relying on photonic entanglement. Using the retrodictive approach, we analyze the properties of the two-photon POVM that are relevant for quantum protocols exploiting two-photon states and measurements. 
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  2. The theory of sum-frequency generation (SFG) as a two-photon measurement process is used to infer the role of two-photon entanglement in this process, and an experimental setup and preliminary data are presented as a way towards quantifying the dependence of SFG on entanglement.

     
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  3. Quantum entanglement plays a prominent role in both foundational physics and emerging quantum technologies. Light is especially promising as a platform for experimental realizations of high-dimensional entanglement, for which the time-frequency degree of freedom provides a natural encoding. Here, we propose and demonstrate a technique to determine the full quantum state of a pair of photons entangled in the time-frequency domain. Our approach, based on spectral shearing interferometry, is entirely self-referenced. To test our system, we measure a photon-pair source with nonlocal spectral phase that results in entanglement between the photons, in which the time when either photon is detected is correlated with the frequency of the other photon. The results demonstrate an effective new tool for exploring the temporal and spectral characteristics of multipartite quantum systems exhibiting high-dimensional entanglement.

     
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  4. Controlling the temporal mode shape of quantum light pulses has wide ranging application to quantum information science and technology. Techniques have been developed to control the bandwidth, allow shifting in the time and frequency domains, and perform mode-selective beam-splitter-like transformations. However, there is no present scheme to perform targeted multimode unitary transformations on temporal modes. Here we present a practical approach to realize general transformations for temporal modes. We show theoretically that any unitary transformation on temporal modes can be performed using a series of phase operations in the time and frequency domains. Numerical simulations show that several key transformations on temporal modes can be performed with greater than 95% fidelity using experimentally feasible specifications.

     
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  5. Single-photon sources are a fundamental resource in quantum optics and quantum information science. Photons with differing spectral and temporal shapes do not interfere well and inhibit the performance of quantum applications such as linear optics quantum computing, boson sampling, and quantum networks. Indistinguishability and purity of photons emitted from different sources are crucial properties for many quantum applications. The ability to determine the state of single-photon sources therefore provides a means to assess their quality, compare different sources, and provide feedback for source tuning. Here, we propose and demonstrate a single-configuration experimental method enabling complete characterization of the spectral-temporal state of a pulsed single-photon source having both pure and mixed states. The method involves interference of the unknown single-photon source with a reference at a balanced beam splitter followed by frequency-resolved coincidence detection at the outputs. Fourier analysis of the joint-spectral two-photon interference pattern reveals the density matrix of the single-photon source in the frequency basis. We present an experimental realization of this method for pure and mixed state pulsed single-photon sources.

     
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  6. Abstract

    Manipulation of quantum optical pulses, such as single photons or entangled photon pairs, enables numerous applications, from quantum communications and networking to enhanced sensing. Common methods to shape laser pulses based upon filtering or amplification cannot be employed with quantum light pulses as these approaches introduce detrimental loss and noise to the system. Here, methods to control and measure quantum light pulses based upon deterministic application of targeted phases in time and frequency domains are reviewed, along with recent demonstrations of quantum applications.

     
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